64gb osmc install

That would also be a good solution, especially with multiple devices. I had tried it a couple of years ago but my NAS was a bit underpowered so I switched back to local cache.

For the OP:

Either edit advancedsettings.xml and add:

<advancedsettings>
 <pathsubstitution>
  <substitute>
    <from>special://thumbnails </from>
    <to>nfs://nas/thumbnails</to>
  </substitute>
 </pathsubstitution>
</advancedsettings>

or edit /etc/fstab and add something like this:

/dev/mmcblk1p1 /home/osmc/.kodi ext4 rw,relatime 0 0